Species we have used to dye wool.
Mushrooms:
Boletus edulis
Hypomyces lactifluorum
Chroogomphus tomentosus
Gomphus clavatus
Paxillus atrotomentosus
Phaeolus schweinitzii
Lichens:
Evernia prunastri
Letharia vulpina
Neprhoma laevigatum
Have you considered the rarer Western Chrysanthemum acea dye? It has a lovely neon orange finish and is slightly velvety to the touch, plus it smells like...well...roses!
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